青藏高原持久性有机污染物的研究进展

摘要/Abstract

摘要：

由于青藏高原特殊的地理条件，对研究持久性有机污染物 (POPs) 的迁移与转化等地球化学过程有着独特的意义。平均海拔高于4 000 m，高山冷凝效应在高原上得到集中体现。大面积的人迹罕至的环境，POPs的分布很少受到人为二次影响。高原地区特有的多冰川的存在，完整地记录了POPs的沉降历史。随着近年来对青藏高原POPs的监测和研究工作的开展，研究者逐渐认识到对高原POPs研究的重要性和认识的不足之处。本研究就目前为止对高原地区POPs的研究现状进行综述，着重介绍对青藏高原不同环境介质中POPs的监测及研究成果，同时总结了高原POPs的物质来源与迁移等研究成果，并根据研究现状提出了展望。

关键词: 青藏高原, 持久性有机污染物, 环境介质, 物质来源

Abstract:

Due to the unique geographical conditions, Tibetan Plateau is an ideal place for researchers to study geochemical processes of persistent organic pollutants (POPs) in natural environment, such as transportation and transformation. The mechanism of mountain cold trapping of POPs could be observed in Tibetan Plateau since its average altitude of more than 4,000 m. The distribution of POPs should rarely be secondly destroyed from few human activities. The precipitation history of POPs could be completely recorded in ices due to so many glaciers in plateau. With research about POPs being done in Tibetan plateau, the importance and significance of the work are gradually recognized. This article intends to review these reports about POPs research so far in plateau area, and focuses on monitoring results in some environmental media. Also, the research results about source and the transportation of POPs are also summarized in this review. In the end, some prospects for future research about POPs in Tibetan Plateau are also proposed.

Key words: Tibetan Plateau, persistent organic pollutant; , environmental media, source

袁国礼, 郎欣欣, 孙天河. 青藏高原持久性有机污染物的研究进展[J]. 现代地质, 2012, 26(5): 910-916.

YUAN Guo-Li, LANG Xin-Xin, SUN Tian-He. A Review of the Research on Persistent Organic Pollutants in Tibetan Plateau[J]. Geoscience, 2012, 26(5): 910-916.

参考文献

[1］岳瑞生.《关于就某些持久性有机污染物采取国际行动的斯德哥尔摩公约》及谈判背景
[J].世界环境，2001(1):24-28.
［2］Hansen J C.Environmental contaminants and human health in the arctic
[J].Toxicology Letters，2000(112/113):119-125.
［3］United Nations Environment Programme. POPS/POPRC.3/5,Distr General
[EB/OL].2007.
[2012-09-12].http://wwwuneporg/.
［4］华小梅，单正军.我国农药的生产、使用状况及其污染环境因子分析
[J].环境科学进展，1996，4(2):30-34.
［5］王晶晶，刘长礼，姜建梅.持久性有机污染物多环芳烃的研究综述
[J].科技创新导报，2010(2)：136-138.
［6］任金亮，王平.多溴联苯醚环境行为的特征与研究进展
[J].化工进展，2006(10)：1152-1157.
［7］Li Y F，Harner T，Liu L，et al.Polychlorinated biphenyls in global air and surface soil: distributions，airsoil exchange，and fractionation effect
[J].Environmental Science & Technology，2010，44:2784-2790.
［8］Wania F，Westgate J.On the mechanism of mountain coldtrapping of organic chemicals
[J].Environmental Science & Technology，2008，42:9092-9098.
［9］Larsson P，Jarnmark C，Sodergren A.PCBs and chlorinated pestieides in the atmosphere and aquatic organisms of Ross Island，Antarctica
[J].Marine Pollution Bulletin，1992，25:281-287.
［10］Weber K，Goerke H.Organochlorine compounds in fish of the Antarctic Peninsula
[J］.Chemosphere，1996，33:377-392.
［11］龙江平，秦大河.雪冰中微量有机物的环境气候变化记录研究进展
[J].冰川冻土，1997，19(2):186-192.
［12］龙江平，秦大河.雪冰中微量有机物的生物地球化学研究进展
[J].矿物岩石地球化学通报，1995(3):67-68.
［13］康世昌，张强弓.青藏高原大气污染科学考察与检测
[J].自然杂志，2010，32(1):13-19.
［14］Kang S，Mayewski P A，Qin D，et al.Glaciochemical records from a Mt.Everest ice core:relationship to atmospheric circulation over Asia
[J].Atmospheric Environment，2002，36:3351-3361.
［15］Li J，Zhu T，Wang F，et al.Observation of organochlorine pesticides in the air of the Mt.Everest region
[J].Ecotoxicology and Environmental Safety，2006，63:33-41.
［16］Cheng H，Zhang G，Jiang J X，et al.Organochlorine pesticides，polybrominated biphenyl ethers and lead isotopes during the spring time at the Waliguan Baseline Observatory，northwest China:implication for longrange atmospheric transport
[J].Atmospheric Environment，2007，41:4734-4747.
［17］Li J，Lin T，Qi S，et al.Evidence of local emission of organochlorine pesticides in the Tibetan Plateau
[J].Atmospheric Environment，2008，42:7397-7404.
［18］Gong P，Wang X P，Sheng J，et al.Variations of organochlorine pesticides and polychlorinated biphenyls in atmosphere of the Tibetan Plateau:Role of the monsoon system
[J].Atmospheric Environment，2010，44:2518-2523.
［19］Gong P，Wang X P，Yao T.Ambient distribution of particulateand gasphase nalkanes and polycyclic aromatic hydrocarbons in the Tibetan Plateau
[J].Environmental Earth Science，2011，64:1703-1711.
［20］Wang X P，Gong P，Yao T D，et al.Passive air sampling of organochlorine pesticides，Polychlorinated Biphenyls，and polybrominated diphenyl ethers across the Tibetan Plateau
[J].Environmental Science & Technology，2010，44:2988-2993.
［21］Wang P，Zhang Q H，Wang Y W，et al.Altitude dependence of polychlorinated biphenyls(PCB) and polybrominated diphenyl ethers(PBDEs) in surface soil from Tibetan Plateau，China
[J].Chemosphere，2009，76:1498-1504.
［22］Guzzella L，Poma G，Paolis A D，et al.Organic persistent toxic substances in soils，waters and sediments along an altitude in algradientat Mt.Sagarmatha，Himalayas，Nepal
[J].Environmental Pollution，2011，159:2552-2564.
［23］李全莲，武小波.雪冰中持久性有机污染物的研究进展
[J].地球与环境，2008，36(1):8-18.
［24］王峰，朱彤，徐柏青，等.珠穆朗玛峰东绒布冰川新降雪中有机氯农药
[J].中国科学：D辑，2007，37(5):670-675.
［25］李全莲，王宁练，武小波，等.祁连山七一冰川雪冰和冰川融水中正构烷烃和多环芳烃的分布特征及来源研究
[J].冰川冻土，2010，32(4):706-713.
［26］李全莲，王宁练，武小波，等.青藏高原冰川雪冰中多环芳烃的分布特征及其来源研究
[J].中国科学:D辑，2010，40(10):1399-1409.
［27］Wang X P，Xu B Q，Kang S C，et al.The historical residue trends of DDT，hexachlorocyclohexanes and polycyclic aromatic hydrocarbons in an ice core from Mt.Everest，central Himalayas
[J].China Atmospheric Environment，2008，42:6699-6709.
［28］Wang X P，Gong P，Zhang Q G，et al.Impact of climate uctuations on deposition of DDT and hexachlorocyclohexane in mountain glaciers:Evidence from ice core records
[J].Environmental Pollution，2010，158:375-380.
［29］Kang J H，Choi S D，Park H，et al.Atmospheric deposition of persistent organic pollutants to the East Rongbuk Glacier in Himalayas
[J].Science of the Total Environment，2009，408:57-63.
［30］张伟玲，张干，祁士华，等.西藏错鄂湖和羊卓雍湖水体及沉积物中有机氯农药的初步研究
[J].地球化学，2003，32(4):363-367.
［31］Wang X P，Yang H D，Gong P，et al.One century sedimentary records of polycyclic aromatic hydrocarbons，mercury and trace elements in the Qinghai Lake
[J].Tibetan Plateau Environmental Pollution，2010，158:3065-3070.
［32］Wang X P，Yao T D，Cong Z Y，et al.Distribution of persistent organic pollutants in soil and grasses around Mt.Qomolangma，China
[J]. Archives of Environmental Contamination and Toxicology，2007，52:153-162.
［33］Wang X P，Yao T D，Cong Z Y，et al.Gradient distribution of persistent organic contaminants along northern slope of centralHimalayas，China
[J].Science of the Total Environment，2006，372:193-202.
［34］Yang R Q，Yao T D，Xu B Q，et al.Distribution of organochlorine pesticides (OCPs) in conifer needles in the southeast Tibetan Plateau
[J].Environmental Pollution，2008，153:92-100.
［35］Wang Y W，Yang R Q，Wang T，et al.Assessment of polychlorinated biphenyls and polybrominated diphenyl ethers in Tibetan butter
[J].Chemosphere，2010，78:772-777.
［36］Chen D，Liu W，Liu X，et al.Coldtrapping of persistent organic pollutions in mountain soils of western Sichuan，China
[J].Environmental Science & Technology，2008，42：9086-9091.

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