Metallogenic Characteristics in the Abrupt Change Zone of Tectono-physicochemical Parameters in the Dayin’gezhuang Gold Orefield,Jiaodong Peninsula

doi:10.19657/j.geoscience.1000-8527.2024.083

Abstract

Abstract:

In the study of orefields with endogenetic metallogenesis,tectono-deformation lithofacies can not only reflect the characteristics of tectonic stress field during the formation of the deposit but also reveal their geoche-mical features and physicochemical conditions.The Jiaodong gold-concentration area has a unique characteristic among global gold deposits,with its scale of gold reserves ranking third in the world.It is noteworthy that the Dayin’gezhuang orefield is one of the super-large gold fields in this region.Based on previous research on tectonic alteration lithofacies,it is particularly necessary to clarify the relationship among the tectono-physicoche-mistry parameters and to delve into how tectonic processes can drive gold mineralization by influencing the physicochemical conditions of ore formation.This study selected tectono-physicochemical parameters representing the composition,temperature and pressure,properties of ore-forming fluids,and conditions of ore-forming structures in order to analyze tectonic diagenesis and mineralization.The results show that the tectono-physicochemistry conditions represented by fluid inclusion components such as CO₂/H₂O,pH,oxygen fugacity (lg$f_{0_{2}}$),tectonic additional hydrostatic pressure (P_s),homogenization temperature of fluid inclusion,minimum pressure of fluid inclusion (P_min),and other parameters have a significant influence on ore formation.The effect of the ore-forming fluid’s composition,properties,temperature and pressure conditions,and the tectonic process represented by CO₂/H₂O,lg$f_{0_{2}}$,P_s,homogenization temperature,and P_min are positively correlated,while the effect of pH shows a negative correlation; additionally,in the pyrite-sericite zone,the pyritic-sericitic granitic cataclastic zone,and the strong potassic feldspar granite belt of the ore field,the tectonic additional hydrostatic pressure (P_s),fluid inclusion component CO₂/H₂O,oxygen fugacity (lg$f_{0_{2}}$),minimum pressure of fluid inclusion (P_min),and homogenization temperature of fluid inclusions exhibit a trend of initially increasing and then decreasing.The ore-forming physical and chemical conditions represented by fluid inclusion component Na⁺/K⁺ and F^-/Cl^- have a negative correlation with ore formation.In the pyrite-sericite zone,pyritic-sericitic granitic cataclastic zone,and strong potassic feldspar granite belt,F^-/Cl^-demonstrate a gradually downward trend,while Na⁺/K⁺ exhibits the opposite trend.Tectonic additional hydrostatic pressure (P_s) can drive ore-forming fluids to migrate from areas with higher P_s to lower P_s,leading to ore precipitation.There is a tectono-physicochemistry interface between the high and low values of tectono-physicochemical parameters,with gold deposits primarily located in stress relaxation zones at this interface.

Key words: tectonic alteration lithofacies, tectono-physicochemical parameter, abrupt change zone, Dayin’gezhuanggold orefield

CLC Number:

P618.51
P613

WANG Zongyong, LÜ Guxian, ZHANG Baolin, LI Yongwu, MA Shengming, HAN Xin, ZHANG Liangliang, YUAN Yuelei, LIU Zhifang, HE Changcheng. Metallogenic Characteristics in the Abrupt Change Zone of Tectono-physicochemical Parameters in the Dayin’gezhuang Gold Orefield,Jiaodong Peninsula[J]. Geoscience, 2024, 38(04): 1043-1053.

Figures/Tables 14

Fig.1 Geological sketch of the Dayin’gezhuang gold ore field(modified from refs.[8-9])

Fig.2 Schematic diagram of tectonic alteration zoning in the Dayin’gezhuang gold ore field (modified after reference [11])

Table 1 Geological characteristics of tectonic alteration zoning in the Dayin’gezhuang gold ore field

构造蚀变分带	岩石颜色	构造	结构	矿物
黄铁绢英岩化带	灰绿色	斑杂状或块状	显微鳞片状花岗变晶结构	石英(30%~35%)、绢云母(25%~30%)、长石(20%~25%)、方解石(5%~10%)和黄铁矿(0.5%~5%)等
黄铁绢英岩化花岗质碎裂岩带	浅灰绿色夹淡肉红色	斑杂状或块状	变余花岗结构、碎裂结构	斜长石(30%±)、钾长石(20%~25%)、石英(25%~30%)、绢云母(10%~15%)和黄铁矿(2%~3%)
强钾长石化花岗岩带	肉红色-浅灰色	块状	花岗结构	钾长石、斜长石、石英、高岭土、绿泥石及星点状黄铁矿,长石、石英含量超过80%
弱钾长石化花岗岩带	灰白色	块状、似片麻状	花岗结构	花岗岩原岩的矿物

Fig.3 Hand specimen and microscopic characteristics of tectonic alteration rocks in the Dayin’gezhuang gold field [11]

Table 2 Parameters of tectono-physicochemistry in the Dayin’gezhuang gold ore field

影响成矿的条件	构造物理化学参量
构造	构造附加静水压力(P_s)
流体	流体包裹体温压	流体包裹体均一温度、
	流体包裹体温压	流体包裹体最小压力(P_min)
	流体包裹体成分	F^-/Cl^-
		Na⁺/K⁺
		CO₂/H₂O
	成矿流体性质	酸碱度(pH)
	成矿流体性质	氧逸度(lg $f O 2$ )
矿化		Au品位

Table 2 Parameters of tectono-physicochemistry in the Dayin’gezhuang gold ore field

影响成矿的条件	构造物理化学参量
构造	构造附加静水压力(P_s)
流体	流体包裹体温压	流体包裹体均一温度、
	流体包裹体温压	流体包裹体最小压力(P_min)
	流体包裹体成分	F^-/Cl^-
		Na⁺/K⁺
		CO₂/H₂O
	成矿流体性质	酸碱度(pH)
	成矿流体性质	氧逸度(lg $f O 2$ )
矿化		Au品位

Table 3 Sample information and methods for obtaining tectono-physicochemical parameters for tectonic alteration zones in the Dayin’gezhuang gold ore field [11]

构造蚀变岩	样品来源	构造物理化学参量获取方法
构造蚀变岩	样品来源	流体包裹体温压	流体包裹体成分	成矿流体性质	构造附加静水压力	金品位
黄铁绢英岩	钻孔岩心	运用LINKAM THMS600型冷热台测试流体包裹体均一温度;根据H₂O-CO₂三相包裹体均一温度等数据,利用FLINCOR程序计算压力	流体包裹体阴阳离子分析采用群体包裹体热爆法,而后用离子色谱法进行测试,部分数据据文献[12]等。流体包裹体气相成分CO₂、H₂O数据据文献[13]、[14]等	pH值和氧逸度(lg $f O 2$ )值据文献[15]、[16]等相关程序计算得出	涉及的变形岩石构造变形比通过Straindesk1.1软件测算;位错密度通过北京大学高倍透射电子显微镜实验中心LBS-2离子减薄仪和日立H9000透射电子显微镜进行观测并计算	Au品位数据据文献[12]等
黄铁绢英岩化花岗质碎裂岩	钻孔岩心
强钾长石化花岗岩	钻孔岩心

Table 3 Sample information and methods for obtaining tectono-physicochemical parameters for tectonic alteration zones in the Dayin’gezhuang gold ore field [11]

构造蚀变岩	样品来源	构造物理化学参量获取方法
构造蚀变岩	样品来源	流体包裹体温压	流体包裹体成分	成矿流体性质	构造附加静水压力	金品位
黄铁绢英岩	钻孔岩心	运用LINKAM THMS600型冷热台测试流体包裹体均一温度;根据H₂O-CO₂三相包裹体均一温度等数据,利用FLINCOR程序计算压力	流体包裹体阴阳离子分析采用群体包裹体热爆法,而后用离子色谱法进行测试,部分数据据文献[12]等。流体包裹体气相成分CO₂、H₂O数据据文献[13]、[14]等	pH值和氧逸度(lg $f O 2$ )值据文献[15]、[16]等相关程序计算得出	涉及的变形岩石构造变形比通过Straindesk1.1软件测算;位错密度通过北京大学高倍透射电子显微镜实验中心LBS-2离子减薄仪和日立H9000透射电子显微镜进行观测并计算	Au品位数据据文献[12]等
黄铁绢英岩化花岗质碎裂岩	钻孔岩心
强钾长石化花岗岩	钻孔岩心

Table 4 Statistics of tectono-physicochemical parameters for tectonic alteration zones in the Dayin’gezhuang gold ore field [11]

构造蚀变岩	CO₂/ H₂O	Au 品位	pH	lg $f O 2$	Na⁺/ K⁺	F^-/ Cl^-	P_s (MPa)	均一温度(℃)	P_min (MPa)
黄铁绢英岩	0.049987	1.16	4.76	-17.633	1.20383	1.403846	94.95	158	212
	0.056471	1.02	4.71	-17.609	1.52391	1.262890	94.85	240	240
	0.050794	0.95	4.75	-16.591	1.35387	1.321257	94.40	251	235
黄铁绢英岩化花岗质碎裂岩	0.110299	0.157	4.70	-13.300	4.197368	1.046653	104.5925	238	253
	0.094167	0.207	4.68	-14.083	3.628349	1.171294	98.5910	278	261
	0.108634	0.139	4.74	-13.937	3.892751	1.118648	101.1020	263	258
	0.118361	0.137	4.61	-14.507	3.936186	1.071541	102.4560	251	256
强钾长石化花岗岩	0.061108	0.051	4.77	-17.633	10.38462	0.421	93.834	148	220
	0.059754	0.086	4.80	-16.851	8.810476	0.592	93.016	276	250
	0.075081	0.069	4.70	-17.902	9.577541	0.616	91.930	229	237

Table 4 Statistics of tectono-physicochemical parameters for tectonic alteration zones in the Dayin’gezhuang gold ore field [11]

构造蚀变岩	CO₂/ H₂O	Au 品位	pH	lg $f O 2$	Na⁺/ K⁺	F^-/ Cl^-	P_s (MPa)	均一温度(℃)	P_min (MPa)
黄铁绢英岩	0.049987	1.16	4.76	-17.633	1.20383	1.403846	94.95	158	212
	0.056471	1.02	4.71	-17.609	1.52391	1.262890	94.85	240	240
	0.050794	0.95	4.75	-16.591	1.35387	1.321257	94.40	251	235
黄铁绢英岩化花岗质碎裂岩	0.110299	0.157	4.70	-13.300	4.197368	1.046653	104.5925	238	253
	0.094167	0.207	4.68	-14.083	3.628349	1.171294	98.5910	278	261
	0.108634	0.139	4.74	-13.937	3.892751	1.118648	101.1020	263	258
	0.118361	0.137	4.61	-14.507	3.936186	1.071541	102.4560	251	256
强钾长石化花岗岩	0.061108	0.051	4.77	-17.633	10.38462	0.421	93.834	148	220
	0.059754	0.086	4.80	-16.851	8.810476	0.592	93.016	276	250
	0.075081	0.069	4.70	-17.902	9.577541	0.616	91.930	229	237

Table 5 Correlation coefficient matrix of variables [11]

		CO₂/H₂O	Au	pH	lg $f O 2$	Na⁺/ K⁺	F^-/ Cl^-	P_s (MPa)	均一温度 (℃)	P_min (MPa)
CO₂/H₂O	皮尔逊相关性	1
	显著性(双尾)
	个案数	10
Au	皮尔逊相关性	-0.611	1
	显著性(双尾)	0.060
	个案数	10	10
pH	皮尔逊相关性	-0.696^*	0.187	1
	显著性(双尾)	0.025	0.605
	个案数	10	10	10
lg $f O 2$	皮尔逊相关性	0.876^**	-0.412	-0.486	1
	显著性(双尾)	0.001	0.237	0.155
	个案数	10	10	10	10
Na⁺/K⁺	皮尔逊相关性	-0.021	-0.752^*	0.251	-0.270	1
	显著性(双尾)	0.954	0.012	0.485	0.450
	个案数	10	10	10	10	10
F^-/Cl^-	皮尔逊相关性	0.042	0.734^*	-0.267	0.279	-0.991^**	1
	显著性(双尾)	0.909	0.016	0.456	0.435	0.000
	个案数	10	10	10	10	10	10
P_s(MPa)	皮尔逊相关性	0.882^**	-0.291	-0.587	0.932^**	-0.350	0.339	1
	显著性(双尾)	0.001	0.414	0.075	0.000	0.322	0.338
	个案数	10	10	10	10	10	10	10
均一温度(℃)	皮尔逊相关性	0.427	-0.261	-0.297	0.537	-0.166	0.169	0.366	1
	显著性(双尾)	0.219	0.467	0.404	0.110	0.646	0.640	0.298
	个案数	10	10	10	10	10	10	10	10
P_min (MPa)	皮尔逊相关性	0.759^*	-0.526	-0.491	0.791^**	-0.061	0.063	0.661^*	0.891^**	1
	显著性(双尾)	0.011	0.118	0.150	0.006	0.866	0.863	0.038	0.001
	个案数	10	10	10	10	10	10	10	10	10

Table 5 Correlation coefficient matrix of variables [11]

		CO₂/H₂O	Au	pH	lg $f O 2$	Na⁺/ K⁺	F^-/ Cl^-	P_s (MPa)	均一温度 (℃)	P_min (MPa)
CO₂/H₂O	皮尔逊相关性	1
	显著性(双尾)
	个案数	10
Au	皮尔逊相关性	-0.611	1
	显著性(双尾)	0.060
	个案数	10	10
pH	皮尔逊相关性	-0.696^*	0.187	1
	显著性(双尾)	0.025	0.605
	个案数	10	10	10
lg $f O 2$	皮尔逊相关性	0.876^**	-0.412	-0.486	1
	显著性(双尾)	0.001	0.237	0.155
	个案数	10	10	10	10
Na⁺/K⁺	皮尔逊相关性	-0.021	-0.752^*	0.251	-0.270	1
	显著性(双尾)	0.954	0.012	0.485	0.450
	个案数	10	10	10	10	10
F^-/Cl^-	皮尔逊相关性	0.042	0.734^*	-0.267	0.279	-0.991^**	1
	显著性(双尾)	0.909	0.016	0.456	0.435	0.000
	个案数	10	10	10	10	10	10
P_s(MPa)	皮尔逊相关性	0.882^**	-0.291	-0.587	0.932^**	-0.350	0.339	1
	显著性(双尾)	0.001	0.414	0.075	0.000	0.322	0.338
	个案数	10	10	10	10	10	10	10
均一温度(℃)	皮尔逊相关性	0.427	-0.261	-0.297	0.537	-0.166	0.169	0.366	1
	显著性(双尾)	0.219	0.467	0.404	0.110	0.646	0.640	0.298
	个案数	10	10	10	10	10	10	10	10
P_min (MPa)	皮尔逊相关性	0.759^*	-0.526	-0.491	0.791^**	-0.061	0.063	0.661^*	0.891^**	1
	显著性(双尾)	0.011	0.118	0.150	0.006	0.866	0.863	0.038	0.001
	个案数	10	10	10	10	10	10	10	10	10

Table 6 Total variance explained[11]

变量	初始特征值			提取载荷平方和			旋转载荷平方和
变量	总计	方差百分比	累积(%)	总计	方差百分比	累积(%)	总计	方差百分比	累积(%)
CO₂/H₂O	4.604	51.154	51.154	4.604	51.154	51.154	3.051	33.903	33.903
Au	2.755	30.616	81.771	2.755	30.616	81.771	2.742	30.468	64.371
pH	0.965	10.726	92.497	0.965	10.726	92.497	1.917	21.302	85.672
lg $f O 2$	0.569	6.324	98.821	0.569	6.324	98.821	1.166	12.957	98.629
Na⁺/K⁺	0.057	0.628	99.449	0.057	0.628	99.449	0.055	0.609	99.238
F^-/Cl^-	0.033	0.369	99.818	0.033	0.369	99.818	0.050	0.559	99.796
P_s(MPa)	0.014	0.154	99.972	0.014	0.154	99.972	0.015	0.168	99.965
均一温度(℃)	0.002	0.027	99.999	0.002	0.027	99.999	0.003	0.034	99.999
P_min(MPa)	8.676E-5	0.001	100.000	8.676E-5	0.001	100.000	0	0.001	100.000

Table 6 Total variance explained[11]

变量	初始特征值			提取载荷平方和			旋转载荷平方和
变量	总计	方差百分比	累积(%)	总计	方差百分比	累积(%)	总计	方差百分比	累积(%)
CO₂/H₂O	4.604	51.154	51.154	4.604	51.154	51.154	3.051	33.903	33.903
Au	2.755	30.616	81.771	2.755	30.616	81.771	2.742	30.468	64.371
pH	0.965	10.726	92.497	0.965	10.726	92.497	1.917	21.302	85.672
lg $f O 2$	0.569	6.324	98.821	0.569	6.324	98.821	1.166	12.957	98.629
Na⁺/K⁺	0.057	0.628	99.449	0.057	0.628	99.449	0.055	0.609	99.238
F^-/Cl^-	0.033	0.369	99.818	0.033	0.369	99.818	0.050	0.559	99.796
P_s(MPa)	0.014	0.154	99.972	0.014	0.154	99.972	0.015	0.168	99.965
均一温度(℃)	0.002	0.027	99.999	0.002	0.027	99.999	0.003	0.034	99.999
P_min(MPa)	8.676E-5	0.001	100.000	8.676E-5	0.001	100.000	0	0.001	100.000

Table 7 Component matrix[11]

变量	成分
变量	F1	F2	F3	F4	F5	F6	F7
CO₂/H₂O	0.931	-0.186	-0.278	0.013	-0.060	0.131	0.008
Au	-0.459	0.881	0.059	-0.045	0.087	0.015	-0.004
pH	-0.687	-0.137	0.349	0.620	-0.009	0.054	-0.005
lg $f O 2$	0.936	0.049	-0.068	0.313	-0.074	-0.111	0.010
Na⁺/K⁺	-0.226	-0.972	-0.032	-0.042	0.003	-0.001	0.029
F^-/Cl^-	0.235	0.965	0.025	0.026	-0.107	0.024	0.015
P_s(MPa)	0.897	0.152	-0.291	0.247	0.165	0.006	0.021
均一温度(℃)	0.675	-0.002	0.721	-0.139	0.025	0.010	0.064
P_min(MPa)	0.901	-0.159	0.389	-0.049	0.023	0.008	-0.090

Table 7 Component matrix[11]

变量	成分
变量	F1	F2	F3	F4	F5	F6	F7
CO₂/H₂O	0.931	-0.186	-0.278	0.013	-0.060	0.131	0.008
Au	-0.459	0.881	0.059	-0.045	0.087	0.015	-0.004
pH	-0.687	-0.137	0.349	0.620	-0.009	0.054	-0.005
lg $f O 2$	0.936	0.049	-0.068	0.313	-0.074	-0.111	0.010
Na⁺/K⁺	-0.226	-0.972	-0.032	-0.042	0.003	-0.001	0.029
F^-/Cl^-	0.235	0.965	0.025	0.026	-0.107	0.024	0.015
P_s(MPa)	0.897	0.152	-0.291	0.247	0.165	0.006	0.021
均一温度(℃)	0.675	-0.002	0.721	-0.139	0.025	0.010	0.064
P_min(MPa)	0.901	-0.159	0.389	-0.049	0.023	0.008	-0.090

Table 8 Component matrix after rotation[11]

变量	成分
变量	Z1	Z2	Z3	Z4	Z5	Z6	Z7
CO₂/H₂O	0.835	-0.168	0.254	0.419	-0.001	0.187	0.005
Au	-0.415	0.862	-0.232	-0.110	-0.108	-0.084	-0.008
pH	-0.347	-0.110	-0.157	-0.918	-0.004	0.001	-0.002
lg $f O 2$	0.906	0.088	0.363	0.113	0.161	-0.027	0.004
Na⁺/K⁺	-0.163	-0.979	-0.074	-0.082	0.003	0.023	-0.017
F^-/Cl^-	0.161	0.975	0.074	0.101	0.065	0.051	-0.020
P_s(MPa)	0.933	0.167	0.169	0.238	-0.113	-0.063	-0.003
均一温度(℃)	0.185	0.060	0.976	0.080	0.003	0.002	-0.051
P_min(MPa)	0.532	-0.106	0.806	0.208	0.014	0.023	0.108

Table 8 Component matrix after rotation[11]

变量	成分
变量	Z1	Z2	Z3	Z4	Z5	Z6	Z7
CO₂/H₂O	0.835	-0.168	0.254	0.419	-0.001	0.187	0.005
Au	-0.415	0.862	-0.232	-0.110	-0.108	-0.084	-0.008
pH	-0.347	-0.110	-0.157	-0.918	-0.004	0.001	-0.002
lg $f O 2$	0.906	0.088	0.363	0.113	0.161	-0.027	0.004
Na⁺/K⁺	-0.163	-0.979	-0.074	-0.082	0.003	0.023	-0.017
F^-/Cl^-	0.161	0.975	0.074	0.101	0.065	0.051	-0.020
P_s(MPa)	0.933	0.167	0.169	0.238	-0.113	-0.063	-0.003
均一温度(℃)	0.185	0.060	0.976	0.080	0.003	0.002	-0.051
P_min(MPa)	0.532	-0.106	0.806	0.208	0.014	0.023	0.108

Fig.4 Tendency chart of the structural deformation ratio of tectonic alteration rock zones in the Dayin’gezhuang gold ore field (using data from reference[11])

Fig.5 Tendency chart of differential stress values during the metallogenic period of tectonic alteration rock zones in the Dayin’gezhuang gold ore field (using data from reference[11])

Fig.6 Schematic diagram of metallogenic characteristics in the rapid change zone of the tectono-physicochemical parameters in the Dayin’gezhuang gold ore field (modified according to reference[11])

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