Geochemical Characteristics and Sources Identification of Atmospheric  Particles in Southern Song-Nen Plain in Heilongjiang Province

Abstract

Abstract:

Twenty-eight samples of atmospheric particles were collected from the southern area of Song-Nen plain, during the summer of 2008. Both the major and minor element concentrations in the samples were analyzed in this research. This paper shows the mass concentrations, correlations and spatial distributions of the elements. And also, the sources of the various elements were identified by enrichment factors and factor analysis. The results show that the elements which are abundant in PM10-100 particles are those which have high concentrations in the crust. Heavy metals have relatively high concentrations in the PM2-5 particles. Mass concentrations of atmospheric particles decrease as: Daqing > Suihua > Harbin > Qiqihar. The enrichment factors of Fe, K, Ti, Mn and Co are smaller than 1 or very close to 1. As for Ca, Mg, Ni and Cr, the enrichment factors are greater than 1 but still smaller than 10. Whereas the enrichment factors of Na, Zn, Cu, Cd, Pb and Se are greater than 10, indicating these elements have anthropogenic sources. The varimax rotated factor analysis shows that the major source of atmospheric inhalable particles is soil dust. Other sources include coal combustion, garbage incineration, automobile tail gas, alkali dust through atmospheric transmission, fuel combustion and industrial sources.

Key words: atmospheric particle, mass concentration, enrichment factor, principal factor analysis, Song-Nen plain

CLC Number:

X142

WEN Yu-Bo, YANG Zhong-Fang, XIA Xue-Qi, CHENG Xin-Bin. Geochemical Characteristics and Sources Identification of Atmospheric Particles in Southern Song-Nen Plain in Heilongjiang Province[J]. Geoscience, 2010, 24(4): 807-815.

References

［1］魏复盛, 腾恩江, 吴国平, 等. 我国4个大城市空气PM2.5、PM10污染及其化学组成［J］. 中国环境监测, 2001, 17(7): 1-6.
［2］刘泽常, 王志强, 李敏, 等. 大气可吸入颗粒物研究进展［J］. 山东科技大学学报：自然科学版, 2004, 23(4): 97-100.
［3］王淑兰, 柴发合, 杨天行. 北京市不同尺度大气颗粒物元素组成的特征分析［J］. 环境科学研究, 2002, 15(4): 10-15.
［4］He K B, Yang F M, Ma Y, et al. The characteristics of PM2.5 in Beijing, China ［J］. Atmospheric Environment, 2001, 35 : 4959-4970.
［5］杨圣杰, 陈莎, 袁波祥. 北京市25 μm小颗粒大气气溶胶特征及来源［J］. 北京交通大学学报, 2001, 25(6): 50-53.
［6］Wang G, Huang L, Gao S W. Characterization of water-soluble species of PM10 and PM2.5 aerosols in urban area in Nanjing, China ［J］. Atmospheric Environment, 2002, 36: 1299-1307.
［7］董雪玲, 刘大锰, 袁杨森, 等. 北京市大气PM10中有机污染物的分布特征［J］. 现代地质, 2008, 22(2): 325-330.
［8］胡克, 陈兵, Hiroyuki Kitagawa, 等. 松嫩平原西部碱尘气溶胶的元素特征分析［J］. 吉林大学学报：地球科学版, 2006, 36(3): 417-423.
［9］He L Y, Hu M, Huang X F, et al. Seasonal pollution characteristics of organic compounds in atmospheric fine particles in Beijing ［J］. Science of the Total Environment, 2006, 359: 167-176.
［10］陈爱凤, 李基明, 陈晓斌, 等. 黑龙江省主要城市环境空气质量状况和变化趋势分析［J］. 北方环境, 2001, 6(2): 17-19.
［11］Nriagu J O, Pacyna J M. Quantitative assessment of worldwide contamination of air, water, and soils by trace metals ［J］. Nature, 1988, 33: 134-139.
［12］Alloway B J. Heavy Metals in Soils ［M］. London: Blackie Academic and Professional, 1995：230-241.
［13］Pacyna J M. Toxicology of Metals ［M］. Boca Raton: CRC Press, 1996：117-123.
［14］杨复沫, 贺克斌, 马永亮, 等. 北京大气细粒子PM2.5的化学组成［J］. 清华大学学报, 2002, 42(12): 1605-1608.
［15］林治卿, 袭著革, 杨丹凤, 等. 采暖期大气中不同粒径颗粒物污染及其重金属分布状况［J］. 环境与健康杂志, 2005, 22(1): 33-34.
［16］孙珍全, 邵龙义, 黄宇婷, 等. 北京市空气中PM10与PM2.5污染水平状况研究［J］. 北京工业职业技术学院学报, 2006, 19(3): 29-34.
［17］刘大锰, 马永胜, 高少鹏. 北京市区春季燃烧源大气颗粒物的污染水平和影响因素［J］. 现代地质, 2005, 19(4): 627 -633.
［18］Wei F, Teng E, Wu G, et al. Ambient concentrations and elemental composition of PM10 and PM2.5 in four Chinese cities ［J］. Environment Science and Technology, 1999, 33: 4188-4193.
［19］崔玉军, 时永明, 刘国栋, 等. 黑龙江省松嫩平原南部黑土的元素含量特征［J］. 现代地质, 2008, 22(6): 929-933.
［20］杨勇杰, 王跃思, 温天雪, 等. 北京市大气颗粒物中PM10和PM2.5质量浓度及其化学组分的特征分析［J］. 环境化学, 2008, 27(1): 117- 118

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Geochemical Characteristics and Sources Identification of Atmospheric Particles in Southern Song-Nen Plain in Heilongjiang Province

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